My favorite's always been "Island of the Giant Pokémon" because I thought it was cool how they let us know what the Pokémon were actually saying when they talked. I sort of wished they would do that more often.
Also, "Electric Soldier Porygon" - it's so incredibly out there and has a great story.
Also, "Electric Soldier Porygon" - it's so incredibly out there and has a great story.

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